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Order-disorder transition in B-type Cu2ZnSnS4 and limitations of ordering through thermal treatments.

This contribution seamlessly follows up on the ongoing discussion concerning the order‐disorder transition in Kesterite Cu2ZnSnS4 (CZTS). We present a method to quantify the degree of cation order in B‐type CZTS from resonant Raman spectroscopy and explore the limitations of thermal treatments for inducing higher order in B‐type CZTS, based on theoretical considerations.

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